C-H Activation for Sustainable Synthesis: Base Metal- and Electro-Catalysis

by Nicolas Sauermann
Doctoral thesis
Date of Examination:2018-07-03
Date of issue:2018-08-07
Advisor:Prof. Dr. Lutz Ackermann
Referee:Prof. Dr. Lutz Ackermann
Referee:Prof. Dr. Konrad Koszinowski
Persistent Address: http://dx.doi.org/10.53846/goediss-6998

 

 

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Abstract

English

In the recent decades, metal-catalyzed C-H activation greatly expanded the available tools for the sustainable synthesis of bioactive molecules and organic materials. Within this thesis, new synthetic transformations based on C-H activation by earth-abundant and cost-effective cobalt and manganese catalysis were developed. Additionally, new synthetic methods combining metal-catalyzed C-H activation with electrosynthesis were explored, thus greatly increasing the sustainable nature of the oxidative C-H activation approach.
Keywords: C-H Activation; Cobalt Catalysis; Manganese Catalysis; Electrocatalysis; Alkynylation; Oxygenation; Amination
 
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