Charakterisierung von Intermediaten in Cobalt-vermittelten Reaktionen

Kreyenschmidt, Friedrich

dc.contributor.advisor	Koszinowski, Konrad Prof. Dr.
dc.contributor.author	Kreyenschmidt, Friedrich
dc.date.accessioned	2019-04-03T09:48:40Z
dc.date.available	2019-04-03T09:48:40Z
dc.date.issued	2019-04-03
dc.identifier.uri	http://hdl.handle.net/11858/00-1735-0000-002E-E5F7-2
dc.identifier.uri	http://dx.doi.org/10.53846/goediss-7379
dc.identifier.uri	http://dx.doi.org/10.53846/goediss-7379
dc.language.iso	deu	de
dc.publisher	Niedersächsische Staats- und Universitätsbibliothek Göttingen	de
dc.rights.uri	http://creativecommons.org/licenses/by-nc-nd/4.0/
dc.subject.ddc	540	de
dc.title	Charakterisierung von Intermediaten in Cobalt-vermittelten Reaktionen	de
dc.type	doctoralThesis	de
dc.title.translated	Characterization of Intermediates in Cobalt-Mediated Reactions	de
dc.contributor.referee	Koszinowski, Konrad Prof. Dr.
dc.date.examination	2019-01-22
dc.description.abstracteng	Homogeneous catalysis is from outstanding importance for modern chemical synthesis. In addition to palladium- and nickel-based catalyst systems, which are well established for a long time, also cobalt-based catalysts are known to mediate challenging conversions. The mechanistic details of the letter reactions are not understood in detail till now. In this work electrospray-ionization mass spectrometry is used to detect the elusive intermediates in cobalt-catalyzed cross-coupling, C-H-activation, hydrogenation and polymerization reactions to get insight into the relevant mechanistic processes. Gas-phase fragmentation reactions are used to reveal the unimolecular reactivity of the key intermediates.	de
dc.contributor.coReferee	Ackermann, Lutz Prof. Dr.
dc.subject.eng	homogeneous catalysis	de
dc.subject.eng	analytical chemistry	de
dc.subject.eng	mass spectrometry	de
dc.identifier.urn	urn:nbn:de:gbv:7-11858/00-1735-0000-002E-E5F7-2-0
dc.affiliation.institute	Fakultät für Chemie	de
dc.subject.gokfull	Chemie (PPN62138352X)	de
dc.identifier.ppn	1666649929

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Fakultät für Chemie (inkl. GAUSS) [701]

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