Experimental and Computational Studies on Ruthenium- and Manganese-Catalyzed C-H and C-C Activation

Rogge, Torben

dc.contributor.advisor	Ackermann, Lutz Prof. Dr.
dc.contributor.author	Rogge, Torben
dc.date.accessioned	2019-11-07T11:14:40Z
dc.date.available	2019-11-07T11:14:40Z
dc.date.issued	2019-11-07
dc.identifier.uri	http://hdl.handle.net/21.11130/00-1735-0000-0005-1298-B
dc.identifier.uri	http://dx.doi.org/10.53846/goediss-7725
dc.language.iso	eng	de
dc.publisher	Niedersächsische Staats- und Universitätsbibliothek Göttingen	de
dc.rights.uri	http://creativecommons.org/licenses/by-nc-nd/4.0/
dc.subject.ddc	540	de
dc.title	Experimental and Computational Studies on Ruthenium- and Manganese-Catalyzed C-H and C-C Activation	de
dc.type	doctoralThesis	de
dc.contributor.referee	Ackermann, Lutz Prof. Dr.
dc.date.examination	2019-10-30
dc.description.abstracteng	During the last years, transition metal-catalyzed C–H and C–C activation has emerged as a powerful tool for the selective construction of C–C and C–Het bonds. In this context, a detailed mechanistic understanding of these transformations is of paramount importance for the development of novel catalytic systems as well as the improvement of established synthetic procedures. Within this thesis, ruthenium catalysis was employed for meta-C–H functionalizations, decarboxylative alkylations, and oxidative C–H/C–H activations, among others. Furthermore, the mechanisms of these reactions were investigated by means of experimental as well as computational studies. Additionally, protocols for selective C–H and C–C activations using inexpensive manganese as the catalyst were developed.	de
dc.contributor.coReferee	Koszinowski, Konrad Prof. Dr.
dc.contributor.thirdReferee	Alcarazo, Manuel Prof. Dr.
dc.contributor.thirdReferee	Mata, Ricardo Prof. Dr.
dc.contributor.thirdReferee	Stalke, Dietmar Prof. Dr.
dc.contributor.thirdReferee	John, Michael Dr.
dc.subject.eng	Transition Metal Catalysis	de
dc.subject.eng	Reaction mechanism	de
dc.subject.eng	Ruthenium	de
dc.subject.eng	Manganese	de
dc.subject.eng	DFT calculations	de
dc.subject.eng	C-C Activation	de
dc.subject.eng	C-H Activation	de
dc.subject.eng	Reaction Kinetics	de
dc.identifier.urn	urn:nbn:de:gbv:7-21.11130/00-1735-0000-0005-1298-B-1
dc.affiliation.institute	Fakultät für Chemie	de
dc.subject.gokfull	Chemie (PPN62138352X)	de
dc.identifier.ppn	1681454270

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Fakultät für Chemie (inkl. GAUSS) [701]

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