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Earth-Abundant Transition Metal-Catalyzed Electro-Reductive Cross-Electrophile Coupling Reactions and C–H Activation by Cobaltaelectro-Catalysis

dc.contributor.advisorAckermann, Lutz Prof. Dr.
dc.contributor.authorAng, Nate Woon Jie
dc.date.accessioned2021-12-13T12:40:35Z
dc.date.available2021-12-20T00:50:04Z
dc.date.issued2021-12-13
dc.identifier.urihttp://hdl.handle.net/21.11130/00-1735-0000-0008-59C3-8
dc.identifier.urihttp://dx.doi.org/10.53846/goediss-8993
dc.identifier.urihttp://dx.doi.org/10.53846/goediss-8993
dc.language.isoengde
dc.publisherNiedersächsische Staats- und Universitätsbibliothek Göttingende
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/4.0/
dc.subject.ddc540de
dc.titleEarth-Abundant Transition Metal-Catalyzed Electro-Reductive Cross-Electrophile Coupling Reactions and C–H Activation by Cobaltaelectro-Catalysisde
dc.typedoctoralThesisde
dc.contributor.refereeAckermann, Lutz Prof. Dr.
dc.date.examination2021-11-29
dc.description.abstractengWithin the last decades, immense progresses have been made with transition metal-catalyzed cross-electrophile reactions and C–H activation reactions. The merger of electrocatalysis with such powerful methods have further enabled a series of more sustainable synthetical protocols for tackling issues such as, the alarming proliferation of CO2 in the atmosphere and the increased demand for more effective pharmaceuticals. This thesis illustrates the electro-catalytic use of earth-abundant and cost-effective cobalt catalyst through the efficient Carbon Capture and Utilization (CCU) strategy for the carboxylation reactions of allylic chlorides with atmospheric CO2. In addition, nickelaelectro-catalytic thiolation of alkyl bromides with electrophilic thiosulfonates have also been successfully described.de
dc.contributor.coRefereeDas, Shoubhik Prof. Dr.
dc.contributor.thirdRefereeTietze, Lutz Prof. Dr. Dr.
dc.contributor.thirdRefereeStalke, Dietmar Prof. Dr.
dc.contributor.thirdRefereeFrauendorf, Holm Dr.
dc.contributor.thirdRefereeJohn, Michael Dr.
dc.subject.engelectrochemicalde
dc.subject.engcarbon dioxidede
dc.subject.engcarboxylationde
dc.subject.engcobaltde
dc.subject.engnickelde
dc.subject.engC–H activationde
dc.subject.engannulationde
dc.subject.engthiolationde
dc.subject.engtransition metal catalysisde
dc.subject.engsustainablede
dc.identifier.urnurn:nbn:de:gbv:7-21.11130/00-1735-0000-0008-59C3-8-3
dc.affiliation.instituteFakultät für Chemiede
dc.subject.gokfullChemie  (PPN62138352X)de
dc.description.embargoed2021-12-20
dc.identifier.ppn1782065954


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