Sustainable Syntheses of Substituted Heterocycles through Ruthenium- and Palladium-Catalyzed Direct C−H Bond Functionalizations

Kornhaaß, Christoph Frank

dc.contributor.advisor	Ackermann, Lutz Prof. Dr.
dc.contributor.author	Kornhaaß, Christoph Frank
dc.date.accessioned	2014-10-22T09:24:56Z
dc.date.available	2014-10-22T09:24:56Z
dc.date.issued	2014-10-22
dc.identifier.uri	http://hdl.handle.net/11858/00-1735-0000-0023-9911-5
dc.identifier.uri	http://dx.doi.org/10.53846/goediss-4750
dc.identifier.uri	http://dx.doi.org/10.53846/goediss-4750
dc.language.iso	eng	de
dc.publisher	Niedersächsische Staats- und Universitätsbibliothek Göttingen	de
dc.rights.uri	http://creativecommons.org/licenses/by-nc-nd/3.0/
dc.subject.ddc	540	de
dc.title	Sustainable Syntheses of Substituted Heterocycles through Ruthenium- and Palladium-Catalyzed Direct C−H Bond Functionalizations	de
dc.type	doctoralThesis	de
dc.contributor.referee	Ackermann, Lutz Prof. Dr.
dc.date.examination	2014-06-20
dc.description.abstracteng	The research presented within this thesis is focused on the development of new synthetic methods for the construction of heterocyclic frameworks through ruthenium- and palladium-catalyzed direct C–H bond functionalizations. A new palladium-catalyzed direct alkynylation of oxazoles and thiazoles was elaborated using gem-dichloroalkenes as electrophiles. Furthermore a novel isoquinoline-synthesis was developed, based on an alkyne-annulation via ruthenium-catalyzed direct C–H bond functionalizations of oximes. A similar approach was used for a copper-free aerobic alkyne-annulation through ruthenium-catalyzed direct C–H bond functionalizations of benzoic acids resulting in the formation of isocoumarins.	de
dc.contributor.coReferee	Diederichsen, Ulf Prof. Dr.
dc.subject.eng	Catalysis	de
dc.subject.eng	Direct C-H Functionalization	de
dc.subject.eng	Ruthenium-Catalyzed Annulations	de
dc.subject.eng	Heterocycles	de
dc.subject.eng	Palladium-Catalyzed Alkynylations	de
dc.subject.eng	Sustainable Synthesis	de
dc.identifier.urn	urn:nbn:de:gbv:7-11858/00-1735-0000-0023-9911-5-2
dc.affiliation.institute	Fakultät für Chemie	de
dc.subject.gokfull	Chemie (PPN62138352X)	de
dc.identifier.ppn	798942118

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