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A matter of brightness: table-top X-ray generation inside waveguides and X-ray holography with single free-electron laser pulses

dc.contributor.advisorSalditt, Tim Prof. Dr.
dc.contributor.authorVassholz, Malte Julian Udo
dc.date.accessioned2022-03-22T14:55:11Z
dc.date.available2023-03-25T00:50:08Z
dc.date.issued2022-03-22
dc.identifier.urihttp://resolver.sub.uni-goettingen.de/purl?ediss-11858/13942
dc.identifier.urihttp://dx.doi.org/10.53846/goediss-9130
dc.language.isoengde
dc.rightsAttribution-NonCommercial-NoDerivatives 4.0 International*
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/4.0/*
dc.subject.ddc530de
dc.titleA matter of brightness: table-top X-ray generation inside waveguides and X-ray holography with single free-electron laser pulsesde
dc.typedoctoralThesisde
dc.contributor.refereeSalditt, Tim Prof. Dr.
dc.date.examination2021-03-26de
dc.subject.gokPhysik (PPN621336750)de
dc.description.abstractengX-ray microscopy delivers insights into the structure of optically opaque bulk specimens with high spatial resolution. The source brightness poses a limit on the achievable resolution, however. While table-top X-ray sources are readily available but provide only low brightness, large-facility sources, such as synchrotrons and X-ray free-electron lasers (XFEL), generate radiation with high brightness and high coherence, but are not easily accessible. In this work, we report on and experimentally demonstrate a novel table-top X-ray source concept to generate spatially coherent X-rays with high brightness, that are emitted directly into the modes of a waveguide. Our estimate of the achievable gain increase demonstrates a substantial brightness improvement with respect to other table-top X-ray sources. In another set of experiments, we make use of the high peak brilliance of an XFEL to observe transient states of water under extreme conditions. In a pump-probe scheme, an infrared laser pulse generates a plasma after optical breakdown to seed a cavitation bubble, which we image with a single XFEL pulse. To get access to the pressure distribution within the shockwave of the cavitation bubbles, we calculate the quantitative phase shift based on a tailored phase-retrieval approach. We further complement nanofocus X-ray holography with time-resolved X-ray diffraction to obtain information on the molecular structure of water after dielectric breakdown. This combined approach delivers quantitative information from microscopic to molecular length scales with high temporal resolution.de
dc.contributor.coRefereeRopers, Claus Prof. Dr.
dc.subject.engX-ray microscopyde
dc.subject.engX-ray sourcesde
dc.subject.engphase retrievalde
dc.subject.engwaveguidesde
dc.subject.engpump-probede
dc.subject.engcavitationde
dc.subject.engX-ray diffractionde
dc.subject.engfree-electron laserde
dc.identifier.urnurn:nbn:de:gbv:7-ediss-13942-9
dc.affiliation.instituteFakultät für Physikde
dc.description.embargoed2023-03-25de
dc.identifier.ppn1797016636


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