Chelation-Assisted C–H Activation by Ruthenium and Osmium Catalysts and Recyclable Hybrid Catalysts
von Isaac Choi
Datum der mündl. Prüfung:2021-09-24
Erschienen:2021-10-25
Betreuer:Prof. Dr. Lutz Ackermann
Gutachter:Prof. Dr. Lutz Ackermann
Gutachter:Prof. Dr. Shoubhik Das
Gutachter:Prof. Dr. Manuel Alcarazo
Gutachter:Prof. Dr. Johannes C. L. Walker
Gutachter:Dr. Michael John
Gutachter:Dr. Daniel Janßen-Müller
Dateien
Name:Dissertation_Isaac_Choi_eDiss.pdf
Size:38.8Mb
Format:PDF
Zusammenfassung
Englisch
Since hydrocarbons are omnipresent structural units in organic compounds, the utilization of C–H bonds of hydrocarbons has great potential. Thereby, organic chemists have had utmost interests in the transformation of hydrocarbons to useful and high-valued compounds by straightforward and sustainable methods. In this thesis, C–H activation reactions using representative metals, including ruthenium, osmium, manganese, and copper are described. Beyond the homogeneous realm, recyclable hybrid metal-catalyzed C–H activation approaches are also presented.
Keywords: C–H activation; Ruthenium catalysis; Osmium catalysis; Manganese catalysis; Copper catalysis; Homogeneous catalysis; Heterogeneous catalysis; Hybrid catalysis